How do I change the columns I can "view by" in card view?

I am trying to sort in card view based on the employee(s) assigned to a task. I have a contact list column with this information in GridView. The "view by" feature shows a ton of columns that aren't relevant to how i want to sort but I can't figure out how to switch them out for more columns that are more relevant to my needs. Is this possible?

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